Dynamic hydrogen-intensified methanation of synthetic by-product gases from steelworks

نویسندگان

چکیده

Steelworks' by-product gases contain significant amounts of carbonaceous species, which can serve as carbon source for Power-to-Gas processes. The COx components from the are converted into methane together with renewable hydrogen in a hydrogen-intensified synthesis reaction. Dynamic operation modes methanation discussed to supersede large gas buffer capacities. This paper presents results two-stage concept operated steel industries. first reactor is designed heat pipe cooled structured fixed-bed reactor. Both influence volume flow rate and stoichiometric ratio examined different steady-state operating points well dynamic repetitive alteration those two parameters. provides consistent product quality over wide syngas power range at slightly over-stoichiometric conditions both conditions. Full yield achieved. design allows step changes up 1.6 kW. Catalyst deactivation by coking took place stage during performed experiments. happened probably due unfavourable formation regime while methanizing CO-rich gases.

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ژورنال

عنوان ژورنال: Fuel Processing Technology

سال: 2021

ISSN: ['1873-7188', '0378-3820']

DOI: https://doi.org/10.1016/j.fuproc.2020.106701